Hmmm, to be honest, you've kind of hit the limit of the CPC's tape-as-music-source abilities...
The absolutely best you can ever get is easy to determine - play an audio tape in the 464 tape deck and listen to the mangled mess you get from effectively having a comparator and deciding whether the bit is 1 or 0 from that.
You can get much better results out from the tape deck by outputting PWM, but to read PWM you'd need a sigma-delta ADC in the tape deck instead of an op-amp.